SESS Report 2021 The State of Environmental Science in Svalbard - an annual report

Executive Summary The State of Environmental Science in Svalbard (SESS) report 2021 together with its predecessors contributes to the documentation of the state of the Arctic environment in and around Svalbard, and highlights research conducted within the Svalbard Integrated Arctic Earth Observing System (SIOS). Climate change is a global problem, but many of its impacts are being felt most strongly in the Arctic. Given its remote but accessible location, Svalbard constitutes an ideal place to study the Arctic environment in general, including, more specifically, the causes and consequences of climate change. The Arctic Climate Change Update (2021) emphasised the severity of global climate change for ecosystems across the Arctic. They are undergoing radical changes regarding their structure and functioning, affecting flora, fauna and livelihoods of Arctic communities. Oceanic ecosystems and food webs are directly and indirectly altered by the warming and freshening of the Arctic Ocean. A prolonged open water period and the expansion of open water areas caused by declining sea ice affect under-ice productivity and diversity. These changes have cascading effects through ecosystems and impact the distribution, abundance and seasonality of a variety of marine species. Svalbard is located at one of the key oceanic gateways to the Arctic. This land–ice–ocean transition zone is a system particularly vulnerable to environmental changes. Svalbard’s environment is influenced by maritime processes; thus extensive observation of the ocean system is nowadays necessary. The chapter on the iMOP project reports seawater temperature and salinity variability over the last decades and indicates changes of Svalbard fjord seawater properties. The chapter highlights the role of a collaborative and supportive network of observatory operators and encourages joint planning and maintenance of future marine observatories. Arctic vegetation plays a key role in land–atmosphere interactions. Alterations can lead to ecosystem–climate feedbacks and exacerbate climate change. Extreme precipitation events are already becoming more frequent. Together with an increasing rain-to-snow ratio they impact the structure and functioning of terrestrial ecosystems. Dynamics in Arctic tundra ecosystems are expected to undergo fundamental changes with increasing temperatures as predicted by climate models. To detect, document, understand and predict those changes, COAT Svalbard provides a long-term and real-time operational observation system through ecosystem-based terrestrial monitoring. The observation system consists of six modules comprising food web pathways as well as one climate-monitoring module and focuses on two contrasting regions in Svalbard to allow for intercomparison. To date, the project has done an initial assessment of tundra ecosystems in Norway and will now begin with the long-term ecosystembased monitoring. For remote regions such as the Svalbard archipelago, terrestrial photography is a crucial addition to satellite imagery, because land-based cameras offer high temporal resolution and insensitivity towards varying weather conditions. PASSES provides an overview of cameras operating in Svalbard managed by research institutions and private companies. The survey revealed difficulties and knowledge gaps preventing the full potential of the terrestrial photography network in Svalbard from being used. Therefore, PASSES recommends the creation of a Svalbard camera system network. The effects of climate change contributed to a specific anomaly of the springtime Arctic atmosphere, namely a pronounced depletion of stratospheric ozone during March and April 2020, which can be called an Arctic ozone hole. In Svalbard, the amount of ozone loss was recorded by ground-based dedicated spectroscopic instruments measuring the total ozone column as well as the UV irradiance (EXAODEP-2020, an update of UV Ozone). The latter is important for effects on the biota. Corresponding erythemal daily doses for spring 2020 show a doubling compared to previous years with less or no ozone depletion. While the correspondence between ozone loss and increase in UV doses follows a well-known relationship, the possible later consequences of the observed springtime increase of UV doses on Svalbard’s environment need to be further studied. A particular method to observe the Svalbard environment, which has seen a very strong increase in usage during recent years, is the application of unmanned airborne or marine vehicles. The update on recent publications using these devices (UAV Svalbard) reveals that especially conventional remotely operated aerial vehicles (drones) with camera equipment are now widely used. It is recommended to SIOS to foster interdisciplinary communication among the multitude of drone users to establish exchange of information and data. New EU regulations for drone operations are being put in place from 2022 onwards also in Svalbard. Climate services are receiving more and more attention from Arctic countries, because they translate data into relevant and timely information, thereby supporting governments, societies and industries in planning and decision-making processes. SIOS contributes to climate services by providing research infrastructure with an overarching goal to develop and maintain a regional observational system for long-term measurements in and around Svalbard. The SIOS Core Data (SCD) consists of a list of essential Earth System Science variables relevant to determine environmental change in the Arctic. SCD is developed to improve the relevance and availability of scientific information addressing ESS topics for decision-making. SIOS Core Data providers have committed to maintain the observations for at least five years, to make the data publicly available, and to follow advanced principles of scientific data management and stewardship. Arctic climate change is posing risks to the safety, health and well-being of Arctic communities and ecosystems. Still, there remain gaps in our understanding of physical processes and societal implications. The authors of the SESS chapters have highlighted some unanswered questions and suggested concrete actions that should be taken to address them. The editors would like to thank the authors for their valuable contributions to the SESS Report 2021. These chapters illustrate how SIOS projects contribute to ensure the future vitality and resilience of Arctic peoples, communities and ecosystems

Effect of addition of four base compounds on sulphuric-acid–water new-particle formation : a laboratory study

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An extensive data set for in situ microphysical characterization of low-level clouds in a Finnish sub-Arctic site

Continuous, semi-long-term, ground-based in situ cloud measurements were conducted during eight Pallas Cloud Experiments (PaCEs) held in autumn between 2004 and 2019. Those campaigns were carried out in the Finnish sub-Arctic region at the Sammaltunturi station (67 degrees 58'24"N, 24 degrees 06'58"E; 560ma.m.s.l.), the part of the Pallas Atmosphere-Ecosystem Supersite and Global Atmosphere Watch (GAW) program. Two cloud spectrometer ground setups and a weather station were installed on the roof of the station to measure in situ cloud properties and several meteorological variables. Thus, the obtained data sets include the size distribution of cloud droplets as a measured cloud parameter along with the air temperature, dew point temperature, humidity, pressure, horizontal wind speed and direction, (global solar) sun radiation, and visibility at the station. Additionally, the number concentration, effective diameter, median volume diameter, and liquid water content from each instrument were derived. The presented data sets provide a insight into microphysics of low-level clouds in subArctic conditions over a wide range of temperatures (-25.8 to 8.8 degrees C). The data are available in the Finnish Meteorological Institute (FMI) open data repository for each campaign and each cloud spectrometer ground setup individually: https://doi.org/10.23728/FMI-B2SHARE.988739D21B824C709084E88ED6C6D54B (Doulgeris et al., 2021).Peer reviewe

Mobile Aerosol Measurement in the Eastern Mediterranean – A Utilization of Portable Instruments

Air pollution research and reports have been limited in the Middle East, especially in Jordan with respect to aerosol particle number concentrations. In this study, we utilized a simple "mobile setup" to measure, for the first time, the spatial variation of aerosol concentrations in Eastern Mediterranean. The mobile setup consisted of portable aerosol instruments to measure particle number concentrations (cut off sizes 0.01, 0.02, 0.3, 0.5, 1, 2.5, 5, and 10 mu m), particle mass concentrations (PM1, PM2.5, and PM10), and black carbon concentration all situated on the back seat of a sedan car. The car was driven with open windows to ensure sufficient cabin air ventilation for reliable outdoor aerosol sampling. Although the measurement campaign was two days long, but it provided preliminary information about aerosols concentrations over a large spatial scale that covered more than three quarters of Jordan. We should keep in mind that the presented concentrations reflect on road conditions. The submicron particle concentrations were the highest in the urban locations (e.g., Amman and Zarqa) and inside cities with heavy duty vehicles activities (e.g., Azraq). The highest micron particle concentrations were observed in the southern part of the country and in places close to the desert area (e.g., Wadi Rum and Wadi Araba). The average submicron concentration was 4.9 x 10(3)-120 x 10(3) cm-3 (5.7-86.7 mu g m(-3)) whereas the average micron particle concentration was 1-11 cm(-3) (8-150 mu g m(-3), assume rho(p) = 1 g cm(-3)). The main road passing through Jafr in the eastern part of Jordan exhibited submicron concentration as low as 800 cm(-3). The PM10 concentration consisted of about 40-75% as PM1. The black carbon (BC) concentration variation was in good agreement with the PM1 as well as the submicron particle number concentration.Peer reviewe

Deterioration of air quality across Sweden due to transboundary agricultural burning emissions

Targino, A. C., Krecl, P., Johansson, C., Swietlicki, E., Massling, A., Coraiola, G. C. & Lihavainen, H. 2013: Deterioration of air quality across Sweden due to transboundary agricultural burning emissions. Boreal Env. Res. 18: 19-36. We analyzed measurements of aerosol and trace-gas concentrations from sites across Sweden before and during a series of agricultural wildland fires in eastern Europe in spring 2006. During the burning episodes, concentrations of background particulate matter (PM) and trace gases, such as carbon monoxide and ozone, increased, affecting air quality across the country and violating national air quality standards. The European Union PM10 daily limit value of 50 mu g m(-3) was exceeded during the pollution episodes even at the background stations, resulting in a nearly four-fold increase as compared with that in non-episode conditions. In relation to a non-episode period, the concentration rise in the accumulation-mode particles was from 40% at an urban site to 340% at a rural site, causing an increase in total particle number concentrations. The fires also boosted ground-level ozone, increasing concentrations of this pollutant by up to 100% at the background stations, which exceeded national air quality standards. Both elemental (EC) and organic carbon (OC) levels increased, with OC making a larger contribution to the total carbonaceous concentrations during the biomass burning episodes. The large-scale atmospheric circulation determined the strength and timing of the pollution events, with the eastern and northern sectors of Sweden experiencing two pollution pulses, whilst sites in the western and southern sectors were affected by one shorter episode. The results show that regional air quality deteriorated due to the long-range transport of pollutants emitted during agricultural wildfires

Influence of air mass origin on microphysical properties of low-level cloudsin a subarctic environment

In this work, an analysis was performed to investigate how different long-range transport air masses can affect the microphysical properties of low-level clouds in a clean subarctic environment. The cloud measurements included in situ and remote sensing ground-based techniques and were conducted during eight Pallas Cloud Experiments (PaCEs) held in the autumn between 2004 and 2019. Each PaCE was carried out at the Pallas Atmosphere-Ecosystem Supersite, located in the Finnish subarctic region. Two cloud spectrometer ground setups were installed on the roof of the station to measure cloud microphysical properties: the cloud, aerosol and precipitation spectrometer (CAPS) and the forward-scattering spectrometer probe (FSSP). Air mass histories were analyzed using the Lagrangian FLEXible PARTicle dispersion model (FLEXPART) in order to investigate the differences between five distinct source regions ( "Arctic ", "Eastern ", "Southern ", "Western " and "Local "). We observed clear differences in the cloud microphysical properties for the air mass source regions. Arctic air masses were characterized by low liquid water content (LWC), low cloud droplet number concentration (Nc) and comparatively large median volume and effective droplet diameter. The Western region (marine North Atlantic) differed from the Arctic by both higher Nc and LWC. The Eastern region (continental Eurasia) only had a little higher LWC than the Arctic but substantially higher Nc and a smaller droplet diameter. The Southern region (continental Europe) had high Nc and LWC and a very similar droplet diameter to the Eastern region. Finally, the relationship between Nc and droplet size (i.e., the Twomey effect) was characterized for the different source regions, indicating that all region clouds were sensitive to increases in Nc.Peer reviewe

Direct radiative feedback due to biogenic secondary organic aerosol estimated from boreal forest site observations

We used more than five years of continuous aerosol measurements to estimate the direct radiative feedback parameter associated with the formation of biogenic secondary organic aerosol (BSOA) at a remote continental site at the edge of the boreal forest zone in Northern Finland. Our upper-limit estimate for this feedback parameter during the summer period (ambient temperatures above 10 degrees C) was -97 +/- 66 mWm(-2) K-1 (mean +/- STD) when using measurements of the aerosol optical depth (f(AOD)) and -63 +/- 40 mWm(-2) K-1 when using measurements of the 'dry' aerosol scattering coefficient at the ground level (f(sigma)). Here STD represents the variability in f caused by the observed variability in the quantities used to derive the value of f. Compared with our measurement site, the magnitude of the direct radiative feedback associated with BSOA is expected to be larger in warmer continental regions with more abundant biogenic emissions, and even larger in regions where biogenic emissions are mixed with anthropogenic pollution.Peer reviewe